| # | Title | Artist | Length |
|---|
| 1 | Clocks (alternate version — 1970 recording) | Emmylou Harris | 2:48 |
| 2 | The Angels Rejoiced Last Night | Gram Parsons & Emmylou Harris | 2:23 |
| 3 | Country Baptizing (The Old) (1973 live version) | Gram Parsons & Emmylou Harris | 4:03 |
| 4 | Coat of Many Colors | Emmylou Harris | 3:43 |
| 5 | For No One | Emmylou Harris | 3:41 |
| 6 | Ooh Las Vegas | Emmylou Harris | 3:44 |
| 7 | Satan’s Jewel Crown | Emmylou Harris | 3:14 |
| 8 | Tulsa Queen | Emmylou Harris | 4:47 |
| 9 | My Songbird | Emmylou Harris | 3:10 |
| 10 | Green Rolling Hills | Emmylou Harris with Fayssoux Starling | 3:37 |
| 11 | One Paper Kid | Emmylou Harris with Willie Nelson | 2:58 |
| 12 | Sorrow in the Wind | Emmylou Harris | 3:30 |
| 13 | Rough and Rocky | Emmylou Harris | 3:53 |
| 14 | Jordan | Emmylou Harris | 2:10 |
| 15 | Darkest Hour Is Just Before the Dawn | Emmylou Harris | 3:24 |
| 16 | Ashes by Now | Emmylou Harris | 4:31 |
| 17 | How High the Moon | Emmylou Harris | 3:23 |
| 18 | Spanish Johnny | Emmylou Harris | 3:51 |
| 19 | The Last Cheater’s Waltz | Emmylou Harris | 5:36 |
| 20 | Racing in the Streets | Emmylou Harris | 5:32 |
| 21 | Like an Old Fashioned Waltz | Emmylou Harris | 3:21 |
| 22 | The Sweetheart of the Rodeo | Emmylou Harris with Dolly Parton, Linda Ronstadt, Vince Gill & Gail Davies | 3:41 |
| 23 | When I Was Yours | Emmylou Harris | 2:46 |
| 24 | My Father’s House | Emmylou Harris | 4:49 |
| 25 | Bright Morning Stars | Emmylou Harris | 2:33 |
| 26 | When He Calls | Emmylou Harris | 2:44 |
| 27 | Lonely Street | Emmylou Harris | 3:12 |
| 28 | Brand New Dance | Emmylou Harris | 3:27 |
| 29 | Get Up John (live) | Emmylou Harris | 3:14 |
| 30 | If I Could Be There (live) | Emmylou Harris | 3:47 |
| 31 | Ballad of a Runaway Horse | Emmylou Harris | 5:40 |
| 32 | Goin’ Back to Harlan | Emmylou Harris | 4:55 |
| 33 | Sweet Old World | Emmylou Harris | 5:07 |
| 34 | All My Tears (live) | Emmylou Harris | 5:08 |
| 35 | Prayer in Open D (live) | Emmylou Harris | 3:59 |
| 36 | Bang the Drum Slowly | Emmylou Harris | 4:53 |
| 37 | Boy From Tupelo | Emmylou Harris | 3:50 |
| 38 | Lost Unto This World | Emmylou Harris | 4:35 |
| 39 | Man Is an Island | Emmylou Harris | 4:45 |
| 40 | Cup of Kindness | Emmylou Harris | 3:54 |
| 41 | Falling in a Deep Hole | Emmylou Harris | 2:38 |
| 42 | 1917 | Emmylou Harris | 5:22 |
| 43 | Palms of Victory (1978 outtake) | Emmylou Harris | 3:07 |
| 44 | Softly and Tenderly (outtake) | Emmylou Harris | 5:30 |
| 45 | My Dear Companion | Emmylou Harris | 2:56 |
| 46 | Mary Danced With Soldiers | Nitty Gritty Dirt Band | 3:06 |
| 47 | I Don’t Love You Much Do I | Guy Clark | 2:37 |
| 48 | All I Left Behind (demo) | Emmylou Harris | 3:18 |
| 49 | I Remember You | Steve Earle | 2:52 |
| 50 | Golden Ring | Emmylou Harris with Linda Ronstadt and Anna & Kate McGarrigle | 3:59 |
| 51 | Sonny | Emmylou Harris, Dolores Keane & Mary Black | 4:17 |
| 52 | In the Garden (1996 recording) | Emmylou Harris | 2:50 |
| 53 | Love Still Remains | Emmylou Harris | 4:36 |
| 54 | Snake Song | Emmylou Harris | 2:32 |
| 55 | Hobo’s Lullaby | Emmylou Harris | 2:42 |
| 56 | Wondering | Emmylou Harris | 3:03 |
| 57 | Immigrant Eyes | Emmylou Harris | 3:41 |
| 58 | Juanita | Sheryl Crow & Emmylou Harris | 2:40 |
| 59 | She | Pretenders & Emmylou Harris | 4:50 |
| 60 | Sin City | Beck & Emmylou Harris | 4:00 |
| 61 | Wheels | The Seldom Scene | 3:28 |
| 62 | Beyond the Blue | Emmylou Harris & Patty Griffin | 4:33 |
| 63 | First in Line (1990 recording) | Emmylou Harris & John Starling | 3:34 |
| 64 | Highway of Headache (1990 recording) | Emmylou Harris | 3:04 |
| 65 | Alone and Forsaken | Emmylou Harris with Mark Knopfler & His Band | 3:31 |
| 66 | Child of Mine | Emmylou Harris | 3:27 |
| 67 | Heaven Ain’t Ready for You Yet | Emmylou Harris | 3:57 |
| 68 | Wish We Were Back in Missouri | Emmylou Harris | 4:03 |
| 69 | Mama’s Hungry Eyes | Emmylou Harris with Rodney Crowell | 3:42 |
| 70 | Here We Are | Emmylou Harris | 2:54 |
| 71 | Waltz Across Texas Tonight (alternate version — 1993 recording) | Emmylou Harris | 3:44 |
| 72 | Snowin’ on Raton (1990 recording) | Emmylou Harris | 3:42 |
| 73 | Gone (outtake — 1993 recording) | Emmylou Harris | 3:37 |
| 74 | Don’t Let Our Love Die | Emmylou Harris | 3:18 |
| 75 | The Pearl (live at Massey Hall 2001) | Emmylou Harris | 5:19 |
| 76 | Wildwood Flower | Randy Scruggs with Emmylou Harris & Iris DeMent | 3:47 |
| 77 | Love and Happiness | Mark Knopfler | 4:21 |
| 78 | When We’re Gone, Long Gone | Emmylou Harris | 4:02 |
