| # | Title | Artist | Length |
|---|
| 1 | Dragnet / Room 43 | Ray Anthony | 4:54 |
| 2 | I Spy | Earle Hagen | 2:13 |
| 3 | Thinking of Baby | Elmer Bernstein | 3:04 |
| 4 | From Russia With Love | Count Basie | 4:16 |
| 5 | Big Town | Laurindo Almeida & The Danzaneros | 2:44 |
| 6 | Man With the Golden Arm | Billy May | 2:52 |
| 7 | The Untouchables | Nelson Riddle | 2:20 |
| 8 | The James Bond Theme | Leroy Holmes | 4:36 |
| 9 | Mission: Impossible | Billy May | 2:27 |
| 10 | Harlem Nocturne | Spike Jones New Band | 2:28 |
| 11 | Walk on the Wild Side | Si Zentner | 2:36 |
| 12 | Mister Kiss Kiss Bang Bang | Elliott Fisher | 1:52 |
| 13 | The Wild Ones | Lou Busch | 2:29 |
| 14 | Staccato’s Theme | Elmer Bernstein | 2:56 |
| 15 | Search for Vulcan | Leroy Holmes | 2:52 |
| 16 | Peter Gunn Suite | Ray Anthony | 8:34 |
| 17 | The Silencers | Vikki Carr | 2:58 |
| 18 | Music to Be Murdered By | Jeff Alexander feat. Alfred Hitchcock | 5:00 |
| 19 | Walk the Lonesome Night | Renzo Cesana | 2:30 |
