| # | Title | Artist | Length |
|---|
| 1 | Aurora (mono) | The Squires | 2:10 |
| 2 | The Sultan (mono) | The Squires | 2:35 |
| 3 | I Wonder (mono) | The Squires | 2:23 |
| 4 | Mustang (instrumental) (mono) | The Squires | 2:25 |
| 5 | I’ll Love You Forever (mono) | The Squires | 3:24 |
| 6 | (I’m a Man and) I Can’t Cry (mono) | The Squires | 2:34 |
| 7 | Hello Lonely Woman (previously unreleased version) | Neil Young & Comrie Smith | 4:00 |
| 8 | Casting Me Away From You | Neil Young & Comrie Smith | 2:16 |
| 9 | There Goes My Babe | Neil Young & Comrie Smith | 2:27 |
| 10 | Sugar Mountain (previously unreleased demo version) (mono) | Neil Young | 2:43 |
| 11 | Nowadays Clancy Can’t Even Sing (demo version) (mono)- recorded in:
- New York, New York, United States (in 1965-12)
- recording engineer:
- Peter K. Siegel (in 1965-12)
- producer:
- Peter K. Siegel and Neil Young
- guitar:
- Neil Young (in 1965-12)
- vocals:
- Neil Young (in 1965-12)
- recording of:
- Nowadays Clancy Can’t Even Sing (in 1965-12)
- lyricist and composer:
- Neil Young
- publisher:
- Broken Arrow Music, Broken Arrow Music Pub, Co., Campbell Connelly & Co. Ltd., Cotillion, Hipgnosis Side B, Richie Furay Music, Springalo Toones, Springalo‐Cotillion Music, Ten East and Ten‐East Music
| Neil Young | 3:05 |
| 12 | Runaround Babe (mono) | Neil Young | 2:39 |
| 13 | The Ballad of Peggy Grover (mono) | Neil Young | 2:48 |
| 14 | The Rent Is Always Due (mono) | Neil Young | 2:54 |
| 15 | Extra, Extra (mono) | Neil Young | 2:44 |
| 16 | Flying on the Ground Is Wrong (mono) | Neil Young | 3:11 |
| 17 | Burned (mono) | Buffalo Springfield | 2:18 |
| 18 | Out of My Mind (mono) | Buffalo Springfield | 3:09 |
| 19 | Down, Down, Down (previously unreleased version) (mono) | Neil Young | 2:14 |
| 20 | Kahuna Sunset (mono) | Buffalo Springfield | 2:55 |
| 21 | Mr. Soul (mono) | Buffalo Springfield | 2:46 |
| 22 | Sell Out (mono) | Buffalo Springfield | 1:43 |
| 23 | Down to the Wire (mono) | Buffalo Springfield | 2:31 |
| 24 | Expecting to Fly- recording engineer:
- Bruce Botnick (on 1967-05-06)
- engineer:
- Bruce Botnick
- producer:
- Jack Nitzsche and Neil Young
- bass and bass guitar:
- Carol Kaye (on 1967-05-06)
- cor anglais, strings, timpani and vibraphone:
- [unknown] (on 1967-05-06)
- drums (drum set):
- Dewey Martin and Jim Gordon (on 1967-05-06)
- electric piano:
- Jack Nitzsche (on 1967-05-06)
- grand piano:
- Don Randi
- guitar:
- Russ Titelman (on 1967-05-06) and Neil Young (on 1967-05-06)
- harpsichord, harpsichord and piano and piano:
- Don Randi (on 1967-05-06)
- choir vocals:
- Merry Clayton (on 1967-05-06), Brenda Holloway (on 1967-05-06), Patrice Holloway (on 1967-05-06), Gloria Jones (on 1967-05-06), Gloria Jones (on 1967-05-06), Sherlie Matthews (on 1967-05-06) and Gracia Nitzsche (on 1967-05-06)
- vocals:
- Richie Furay and Neil Young (on 1967-05-06)
- strings arranger:
- Jack Nitzsche
- arranger:
- Jack Nitzsche and Neil Young
- phonographic copyright (℗) by:
- Warner Bros. Records Inc.
- recorded at:
- Sunset Sound in Hollywood, Los Angeles, California, United States (on 1967-05-06)
- recording of:
- Expecting to Fly (on 1967-05-06)
- lyricist and composer:
- Neil Young
- publisher:
- Broken Arrow Music, Broken Arrow Music Pub, Co., Hipgnosis Side B, Richie Furay Music, Springalo Toones and Ten‐East Music
| Buffalo Springfield | 3:48 |
| 25 | Slowly Burning (instrumental) | Neil Young | 3:01 |
| 26 | One More Sign | Neil Young | 2:05 |
| 27 | Broken Arrow- recording engineer:
- Tom May (on 1967-08-25), Bill Lazarus (from 1967-09-05 until 1967-09-18) and Jim Messina (from 1967-09-05 until 1967-09-18)
- producer:
- Neil Young
- bass:
- Harvey Newmark (from 1967-08-25 until 1967-09-18)
- bass guitar:
- Bruce Palmer (from 1967-08-25 until 1967-09-18)
- clarinet:
- Jim Horn (from 1967-08-25 until 1967-09-18)
- drums (drum set):
- Hal Blaine (from 1967-08-25 until 1967-09-18) and Dewey Martin (from 1967-08-25 until 1967-09-18)
- guitar:
- Richie Furay (from 1967-08-25 until 1967-09-18), Chris Sarns (from 1967-08-25 until 1967-09-18), Stephen Stills (from 1967-08-25 until 1967-09-18) and Neil Young (from 1967-08-25 until 1967-09-18)
- organ and piano and piano:
- Don Randi (from 1967-08-25 until 1967-09-18)
- background vocals:
- Richie Furay (from 1967-08-25 until 1967-09-18)
- vocals:
- Dewey Martin (from 1967-08-25 until 1967-09-18) and Neil Young (from 1967-08-25 until 1967-09-18)
- arranger:
- Neil Young
- phonographic copyright (℗) by:
- Warner Bros. Records Inc.
- recorded at:
- Columbia Recording Studios in Hollywood, Los Angeles, California, United States (on 1967-08-25) and Sunset Sound in Hollywood, Los Angeles, California, United States (from 1967-09-05 until 1967-09-18)
- recording of:
- Broken Arrow (from 1967-08-25 until 1967-09-18)
- lyricist and composer:
- Neil Young
- publisher:
- Broken Arrow Music Pub, Co., Hipgnosis Side B, Richie Furay Music and Silver Fiddle Music
| Buffalo Springfield | 6:18 |
| 28 | I Am a Child | Buffalo Springfield | 2:19 |